Single-ion magnet behaviour in [U(TpMe2)2I]

Joana T. Coutinho; Maria A. Antunes; Laura C. J. Pereira; Hélène Bolvin; Joaquim Marçalo; Marinella Mazzanti; Manuel Almeida

doi:10.1039/C2DT31421E

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Dalton Transactions

Issue 44, 2012

The international journal for inorganic, organometallic and bioinorganic chemistry

Impact Factor 3.838 48 Issues per Year Indexed in MEDLINE

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Single-ion magnet behaviour in [U(Tp^Me2)₂I]

Joana T. Coutinho,^a Maria A. Antunes,^a Laura C. J. Pereira,^a Hélène Bolvin,^b Joaquim Marçalo,^a Marinella Mazzanti^c and Manuel Almeida*^a

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Unidade de Ciências Químicas e Radiofarmacêuticas, IST/ITN, Instituto Superior Técnico/CFMCUL, P-2686-953 Sacavém, Portugal
E-mail: malmeida@itn.pt ;
Fax: +351 219550117 ;
Tel: +351 219946171

Laboratoire de Chimie et de Physique Quantiques – IRSAMC, Université de Toulouse 3, 118 Route de Narbonne, F-31400 Toulouse, France

Laboratoire de Reconnaissance Ionique et Chimie de Coordination, Service de Chimie Inorganique et Biologique, UMR-E 3 CEA/UJF, FRE3200 CNRS, INAC, CEA-Grenoble, F-38054 Grenoble Cedex 09, France

Dalton Trans., 2012,41, 13568-13571

DOI: 10.1039/C2DT31421E
Received 01 Jul 2012, Accepted 26 Jul 2012
First published online 30 Jul 2012

This article is part of themed collection: Frontier and Perspectives in Molecule-Based Quantum Magnet

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Abstract
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[U(Tp^Me2)₂I] exhibits at low temperatures single molecule magnet (SMM) behaviour comparable to its bipyridine derivative and related single ion U(III) complexes recently reported as SMMs. The trend of variation of the energy barrier for the magnetic relaxation in these compounds is well reproduced by quantum chemistry calculations.

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Joana T. Coutinho
Maria A. Antunes
Laura C. J. Pereira
Hélène Bolvin
Joaquim Marçalo
Marinella Mazzanti
Manuel Almeida

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Single-ion magnet behaviour in [U(TpMe2)2I]

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Single-ion magnet behaviour in [U(Tp^Me2)₂I]