Ligand-based solid solution approach to stabilisation of sulphonic acid groups in porous coordination polymer Zr6O4(OH)4(BDC)6 (UiO-66)

Maw Lin Foo; Satoshi Horike; Tomohiro Fukushima; Yuh Hijikata; Yoshiki Kubota; Masaki Takata; Susumu Kitagawa

doi:10.1039/C2DT31195J

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Dalton Transactions

Issue 45, 2012

The international journal for inorganic, organometallic and bioinorganic chemistry

Impact Factor 3.838 48 Issues per Year Indexed in MEDLINE

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Ligand-based solid solution approach to stabilisation of sulphonic acid groups in porous coordination polymer Zr₆O₄(OH)₄(BDC)₆ (UiO-66)

Maw Lin Foo,^a^b Satoshi Horike,^c^d Tomohiro Fukushima,^c Yuh Hijikata,^c Yoshiki Kubota,^e Masaki Takata^f and Susumu Kitagawa*^a^b^c

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Japan Science and Technology Agency, ERATO, Kitagawa Integrated Pores Project, Kyoto Research Park Bldg #3, Shimogyo-ku, Japan

Institute for Integrated Cell-Material Sciences (WPI-iCeMS), Kyoto University, Yoshida, Sakyo-ku, Japan

Department of Synthetic Chemistry and Biological Chemistry, Graduate School of Engineering, Kyoto University, Katsura, Nishikyo-ku, Japan
E-mail: kitagawa@sbchem.kyoto-u.ac.jp ;
Fax: +81-75-383-2732 ;
Tel: +81-75-383-2733

Japan Science and Technology Agency, PRESTO, 4-1-8 Honcho, Kawaguchi, Japan

Osaka Prefecture University, Japan

Japan Synchrotron Radiation Research Institute/SPring-8 Sayo-gun, Hyogo 679-5198, Japan

Dalton Trans., 2012,41, 13791-13794

DOI: 10.1039/C2DT31195J
Received 04 Jun 2012, Accepted 16 Jul 2012
First published online 17 Jul 2012

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By adopting a ligand-based solid solution approach, the sulphonic acid functional group can be successfully incorporated into a porous coordination polymer with UiO-66 structure type. Zr₆O₄(OH)₄(BDC-SO₃H)_1.1(BDC)_4.9 possesses enhanced heat of adsorption for carbon dioxide and acetone compared to Zr₆O₄(OH)₄(BDC)₆.

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Maw Lin Foo
Satoshi Horike
Tomohiro Fukushima
Yuh Hijikata
Yoshiki Kubota
Masaki Takata
Susumu Kitagawa

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Dalton Transactions

Ligand-based solid solution approach to stabilisation of sulphonic acid groups in porous coordination polymer Zr₆O₄(OH)₄(BDC)₆ (UiO-66)

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Dalton Transactions

Ligand-based solid solution approach to stabilisation of sulphonic acid groups in porous coordination polymer Zr6O4(OH)4(BDC)6 (UiO-66)

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Ligand-based solid solution approach to stabilisation of sulphonic acid groups in porous coordination polymer Zr₆O₄(OH)₄(BDC)₆ (UiO-66)