Reduction and oxidation of SrCoO2.5 thin films at low temperatures

Noriya Ichikawa; Monika Iwanowska; Masanori Kawai; Christophe Calers; Werner Paulus; Yuichi Shimakawa

doi:10.1039/C2DT30317E

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Dalton Transactions

Issue 35, 2012

The international journal for inorganic, organometallic and bioinorganic chemistry

Impact Factor 3.838 48 Issues per Year Indexed in MEDLINE

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Reduction and oxidation of SrCoO_2.5 thin films at low temperatures

Noriya Ichikawa,*^a Monika Iwanowska,^a^b Masanori Kawai,^a Christophe Calers,^a^b Werner Paulus^b^d and Yuichi Shimakawa^a^c

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Institute for Chemical Research, Kyoto University, Gokasho, Uji, Japan
E-mail: nori@scl.kyoto-u.ac.jp ;
Fax: +81-774-38-3118 ;
Tel: +81-774-38-3117

MaMaSELF, Université de Rennes 1, Campus de Beaulieu, Bât 10B, F-35042 Rennes, France

Japan Science and Technology Agency, CREST, Uji 611-0011, Japan

Institut de Chimie Moléculaire et des Matériaux, Université de Montpellier, 2. Place Eugène Bataillon, Bat 15, F-34095 Montpellier, France

Dalton Trans., 2012,41, 10507-10510

DOI: 10.1039/C2DT30317E
Received 13 Feb 2012, Accepted 03 May 2012
First published online 03 May 2012

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Abstract
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Brownmillerite SrCoO_2.5 (010) thin films synthesized by pulsed laser deposition became amorphous when reduced at low temperatures by CaH₂, indicating that the infinite-layer structure with the square planar Co²⁺O₄ configuration is unstable. Ferromagnetic and conducting perovskite SrCoO₃ epitaxial thin films, on the other hand, were obtained topotactically at room temperature by oxidation with NaClO.

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Noriya Ichikawa
Monika Iwanowska
Masanori Kawai
Christophe Calers
Werner Paulus
Yuichi Shimakawa

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