Low-voltage electrochemical CO2 reduction by bacterial voltage-multiplier circuits

Taketo Mogi; Takumi Ishii; Kazuhito Hashimoto; Ryuhei Nakamura

doi:10.1039/C2CC37986D

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Chemical Communications

Issue 38, 2013

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Low-voltage electrochemical CO₂ reduction by bacterial voltage-multiplier circuits

Taketo Mogi,^a Takumi Ishii,^a Kazuhito Hashimoto*^a^b and Ryuhei Nakamura*^a

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Department of Applied Chemistry, School of Engineering, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Japan
E-mail: nakamura@light.t.u-tokyo.ac.jp; ;
Fax: +81-3-5841-1142 ;
Tel: +81-3-5841-7248

ERATO/JST, HASHIMOTO Light Energy Conversion Project, Japan
E-mail: hashimoto@light.t.u-tokyo.ac.jp; ;
Fax: +81-3-5841-1142 ;
Tel: +81-3-5841-7248

Chem. Commun., 2013,49, 3967-3969

DOI: 10.1039/C2CC37986D
Received 05 Nov 2012, Accepted 18 Dec 2012
First published online 19 Dec 2012

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Using the voltage-multiplying circuits of chemolitho-autotrophic Fe-oxidizing bacteria (Mariprofundus ferrooxydans), we describe an integrated bioelectrochemical system that affords simultaneous CO₂ reduction and H₂O oxidation at an external voltage of less than 1.24 V.

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