Maximum hydrogen chemisorption on KL zeolite supported Pt clusters

Christopher Jensen; Doris Buck; Herbert Dilger; Matthias Bauer; Fritz Phillipp; Emil Roduner

doi:10.1039/C2CC37933C

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Chemical Communications

Issue 6, 2013

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Maximum hydrogen chemisorption on KL zeolite supported Pt clusters

Christopher Jensen,^a Doris Buck,^a Herbert Dilger,^a Matthias Bauer,^b Fritz Phillipp^c and Emil Roduner*^a

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Institute of Physical Chemistry, University of Stuttgart, Pfaffenwaldring 55, 70569 Stuttgart, Germany
E-mail: e.roduner@ipc.uni-stuttgart.de ;
Fax: +49 711 68564495 ;
Tel: +49 711 68564490

Fachbereich Chemie, Technische Universität Kaiserslautern, Erwin-Schrödinger-Str. 54, 67663 Kaiserslautern, Germany

Max Planck Institute for Intelligent Systems, Heisenbergstr. 3, 70569 Stuttgart, Germany

Chem. Commun., 2013,49, 588-590

DOI: 10.1039/C2CC37933C
Received 27 Aug 2012, Accepted 21 Nov 2012
First published online 22 Nov 2012

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Platinum clusters supported on KL zeolites were characterized by EPR, HRTEM, and EXAFS. Two kinds of hydrogen chemisorption experiments both result in a saturation value of 2.9 hydrogen atoms per platinum atom, significantly more than that reported so far. A hydrogen coverage-dependent cluster restructuring is suggested.

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Christopher Jensen
Doris Buck
Herbert Dilger
Matthias Bauer
Fritz Phillipp
Emil Roduner

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