Catalytic “triangles”: binding of iron in task-specific ionic liquids

Denis Prodius; Fliur Macaev; Eugenia Stingaci; Vsevolod Pogrebnoi; Valeriu Mereacre; Ghenadie Novitchi; George E. Kostakis; Christopher E. Anson; Annie K. Powell

doi:10.1039/C2CC36741F

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Chemical Communications

Issue 19, 2013

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Catalytic “triangles”: binding of iron in task-specific ionic liquids

Denis Prodius,*^a^b Fliur Macaev,^b Eugenia Stingaci,^b Vsevolod Pogrebnoi,^b Valeriu Mereacre,^a Ghenadie Novitchi,^b^c George E. Kostakis,^d Christopher E. Anson^a and Annie K. Powell*^a^d

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Institute of Inorganic Chemistry, Karlsruhe Institute of Technology, Engesserstrasse 15, 76128 Karlsruhe, Germany
E-mail: annie.powell@kit.edu ;
Fax: +49 721-608-48142 ;
Tel: +49 721-608-42135

Institute of Chemistry of the Academy of Sciences of Moldova, Academiei str. 3, MD-2028 Chisinau, Moldova
E-mail: denis.prodius@kit.edu ;
Fax: +373 22 739722 ;
Tel: +373 22 739954

Laboratoire National des Champs Magnétiques Intenses, CNRS UPR 3228, 25 Rue des Martyrs, Grenoble, France

Institute of Nanotechnology, Karlsruhe Institute of Technology, Hermann-von-Helmholtz Platz 1, 76344 Eggenstein-Leopoldshafen, Germany

Chem. Commun., 2013,49, 1915-1917

DOI: 10.1039/C2CC36741F
Received 16 Sep 2012, Accepted 19 Oct 2012
First published online 22 Oct 2012

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A new class of task-specific ionic liquids (ILs) which contain septuply positively charged {Fe₃^IIIO(RCOO)₆L₃}⁷⁺ triangles has been synthesized and structurally characterized. Such metal-containing ILs can be repeatedly used as alternative catalysts in the synthesis of 2-pyrrolo-3′-yloxindole or the condensation of indoles with various aldehydes.

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Denis Prodius
Fliur Macaev
Eugenia Stingaci
Vsevolod Pogrebnoi
Valeriu Mereacre
Ghenadie Novitchi
George E. Kostakis
Christopher E. Anson
Annie K. Powell

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Chemical Communications

Catalytic “triangles”: binding of iron in task-specific ionic liquids

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