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Issue 92, 2012
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Pyridine synthesis by reactions of allyl amines and alkynes proceeding through a Cu(OAc)2 oxidation and Rh(III)-catalyzed N-annulation sequence

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Abstract

A new methodology has been developed for the synthesis of pyridines from allyl amines and alkynes, which involves sequential Cu(II)-promoted dehydrogenation of the allylamine and Rh(III)-catalyzed N-annulation of the resulting α,β-unsaturated imine and alkyne.

Graphical abstract: Pyridine synthesis by reactions of allyl amines and alkynes proceeding through a Cu(OAc)2 oxidation and Rh(iii)-catalyzed N-annulation sequence

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Publication details

The article was received on 14 Sep 2012, accepted on 03 Oct 2012 and first published on 03 Oct 2012


Article type: Communication
DOI: 10.1039/C2CC36699A
Citation: Chem. Commun., 2012,48, 11334-11336
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    Pyridine synthesis by reactions of allyl amines and alkynes proceeding through a Cu(OAc)2 oxidation and Rh(III)-catalyzed N-annulation sequence

    D. Kim, J. Park and C. Jun, Chem. Commun., 2012, 48, 11334
    DOI: 10.1039/C2CC36699A

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