Tandem catalysis with a bifunctional site-isolated Lewis acid–Brønsted base metal–organic framework, NH2-MIL-101(Al)

Renganathan Srirambalaji; Soonsang Hong; Ramalingam Natarajan; Minyoung Yoon; Raghunandan Hota; Yonghwi Kim; Young Ho Ko; Kimoon Kim

doi:10.1039/C2CC36678A

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Chemical Communications

Issue 95, 2012

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Tandem catalysis with a bifunctional site-isolated Lewis acid–Brønsted base metal–organic framework, NH₂-MIL-101(Al)

Renganathan Srirambalaji,^a Soonsang Hong,^a Ramalingam Natarajan,^a Minyoung Yoon,^a Raghunandan Hota,^a Yonghwi Kim,^a Young Ho Ko^a and Kimoon Kim*^a

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Center for Smart Supramolecules, Department of Chemistry and Division of Advanced Materials Science, Pohang University of Science and Technology, San 31 Hyojadong, Pohang 790-784, Republic of Korea
E-mail: kkim@postech.ac.kr ;
Fax: +82-54-279-8129 ;
Tel: +82-54-279-2113

Chem. Commun., 2012,48, 11650-11652

DOI: 10.1039/C2CC36678A
Received 13 Sep 2012, Accepted 19 Oct 2012
First published online 22 Oct 2012

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A metal–organic framework (MOF), NH₂-MIL-101(Al), which acts as a bifunctional, site-isolated Lewis acid–Brønsted base heterogeneous catalyst, catalyzes a tandem Meinwald rearrangement–Knoevenagel condensation reaction with remarkable substrate selectivity.

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Renganathan Srirambalaji
Soonsang Hong
Ramalingam Natarajan
Minyoung Yoon
Raghunandan Hota
Yonghwi Kim
Young Ho Ko
Kimoon Kim

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Chemical Communications

Tandem catalysis with a bifunctional site-isolated Lewis acid–Brønsted base metal–organic framework, NH₂-MIL-101(Al)

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Tandem catalysis with a bifunctional site-isolated Lewis acid–Brønsted base metal–organic framework, NH2-MIL-101(Al)

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Tandem catalysis with a bifunctional site-isolated Lewis acid–Brønsted base metal–organic framework, NH₂-MIL-101(Al)