PbO2: from semi-metal to transparent conducting oxide by defect chemistry control

Aron Walsh; Aoife B. Kehoe; Douglas J. Temple; Graeme W. Watson; David O. Scanlon

doi:10.1039/C2CC35928F

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Chemical Communications

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PbO₂: from semi-metal to transparent conducting oxide by defect chemistry control

Aron Walsh,*^a Aoife B. Kehoe,^b Douglas J. Temple,^b Graeme W. Watson*^b and David O. Scanlon*^c

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Centre for Sustainable Chemical Technologies and Department of Chemistry, University of Bath, Claverton Down, Bath BA2 7AY, UK
E-mail: a.walsh@bath.ac.uk

School of Chemistry and CRANN, Trinity College Dublin, Dublin 2, Ireland
E-mail: watsong@tcd.ie

University College London, Kathleen Lonsdale Materials Chemistry, Department of Chemistry, 20 Gordon Street, London WC1H 0AJ, UK
E-mail: d.scanlon@ucl.ac.uk

Chem. Commun., 2013,49, 448-450

DOI: 10.1039/C2CC35928F
Received 16 Aug 2012, Accepted 22 Nov 2012
First published online 23 Nov 2012

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Lead dioxide has been studied for over 150 years as a component of the lead-acid battery. Based on first-principles calculations, we predict that by tuning the concentration of electrons in the material, through control of the defect chemistry, PbO₂ can be rendered from black to optically transparent, thus opening up applications in the field of optoelectronics.

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Aoife B. Kehoe
Douglas J. Temple
Graeme W. Watson
David O. Scanlon

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