Chemoenzymatic preparation of germacrene analogues

Oscar Cascón; Sabrina Touchet; David J. Miller; Veronica Gonzalez; Juan A. Faraldos; Rudolf K. Allemann

doi:10.1039/C2CC35542F

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Chemical Communications

Issue 78, 2012

Urgent high quality communications from across the chemical sciences.

Impact Factor 6.169 100 Issues per Year Indexed in MEDLINE

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Chemoenzymatic preparation of germacrene analogues

Oscar Cascón,^a Sabrina Touchet,^a David J. Miller,^a Veronica Gonzalez,^a Juan A. Faraldos^a and Rudolf K. Allemann*^a

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School of Chemistry and Cardiff Catalysis Institute, Cardiff University, Main Building, Park Place, Cardiff CF10 3AT, UK
E-mail: allemannrk@cardiff.ac.uk ;
Fax: +44 (0)29 208 74030 ;
Tel: +44 (0)29 208 79014

Chem. Commun., 2012,48, 9702-9704

DOI: 10.1039/C2CC35542F
Received 31 Jul 2012, Accepted 14 Aug 2012
First published online 15 Aug 2012

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A small library of novel germacrenes was generated using a combination of two plant enzymes, germacrene A synthase, and D synthase and modified farnesyl diphosphate (FDP) analogues. This chemoenzymatic approach allows the preparation of potentially valuable volatiles for biological studies.

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Oscar Cascón
Sabrina Touchet
David J. Miller
Veronica Gonzalez
Juan A. Faraldos
Rudolf K. Allemann

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