Unprecedented CO2 uptake over highly porous N-doped activated carbon monoliths prepared by physical activation

Mahasweta Nandi; Keisuke Okada; Arghya Dutta; Asim Bhaumik; Jun Maruyama; Didi Derks; Hiroshi Uyama

doi:10.1039/C2CC35334B

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Chemical Communications

Issue 83, 2012

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Unprecedented CO₂ uptake over highly porous N-doped activated carbon monoliths prepared by physical activation

Mahasweta Nandi,^a Keisuke Okada,^a Arghya Dutta,^a^b Asim Bhaumik,^b Jun Maruyama,^c Didi Derks^a and Hiroshi Uyama*^a

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Department of Applied Chemistry, Graduate School of Engineering, Osaka University, Yamadaoka 2-1, Japan
E-mail: uyama@chem.eng.osaka-u.ac.jp ;
Fax: +81-6-6879-7367 ;
Tel: +81-6-6879-7364

Department of Materials Science, Indian Association for the Cultivation of Science, Jadavpur, India

Environmental Technology Research Division, Osaka Municipal Technical Research Institute, 1-6-50 Morinomiya, Joto-ku, Japan

Chem. Commun., 2012,48, 10283-10285

DOI: 10.1039/C2CC35334B
Received 24 Jul 2012, Accepted 09 Aug 2012
First published online 09 Aug 2012

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Highly porous N-doped activated carbon monoliths (ACMs) are fabricated by carbonization and physical activation of mesoporous polyacrylonitrile (PAN) monoliths in the presence of CO₂. The monoliths exhibit exceptionally high CO₂ uptake; 5.14 mmol g⁻¹ at ambient pressure and temperature and 11.51 mmol g⁻¹ at ambient pressure and 273 K.

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Mahasweta Nandi
Keisuke Okada
Arghya Dutta
Asim Bhaumik
Jun Maruyama
Didi Derks
Hiroshi Uyama

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Unprecedented CO₂ uptake over highly porous N-doped activated carbon monoliths prepared by physical activation