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Reactions of the [1,2-(NH)2C6H4]2− dianion (LH22−) with Cp2MII (M = V, Mn) lead to complete or partial oxidation of the metals (M), giving the VIII compound [(η5-Cp)(LH2)2VV(LH2)]−[Li(THF)4]+ (1) and MnII4MnIII2 oxo cage [Mn6(LH2)6(μ6-O)(THF)4] (2).
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