Sub-oxide-to-metallic, uniformly-nanoporous crystalline nanowires by plasma oxidation and electron reduction

Uroš Cvelbar; Zhiqiang Chen; Igor Levchenko; R. Michael Sheetz; Jacek B. Jasinski; Madhu Menon; Mahendra K. Sunkara; Kostya (Ken) Ostrikov

doi:10.1039/C2CC35151J

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Chemical Communications

Issue 90, 2012

Urgent high quality communications from across the chemical sciences.

Impact Factor 6.169 100 Issues per Year Indexed in MEDLINE

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Sub-oxide-to-metallic, uniformly-nanoporous crystalline nanowires by plasma oxidation and electron reduction

Uroš Cvelbar,*^a Zhiqiang Chen,^b Igor Levchenko,^c^d R. Michael Sheetz,^e Jacek B. Jasinski,^b Madhu Menon,^e^f Mahendra K. Sunkara^b and Kostya (Ken) Ostrikov^c^d

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Jozef Stefan Institute, Jamova cesta 39, Slovenia
E-mail: uros.cvelbar@ijs.si

CONN Centre for Renewable Research, University of Louisville, Louisville, USA

Plasma Nanoscience Centre Australia (PNCA), CSIRO Materials Science and Engineering, P.O. Box 218, Lindfield, Australia

Plasma Nanoscience, School of Physics, The University of Sydney, Sydney, Australia

Center for Computational Sciences, University of Kentucky, Lexington, USA

Department of Physics and Astronomy, University of Kentucky, Lexington, USA

Chem. Commun., 2012,48, 11070-11072

DOI: 10.1039/C2CC35151J
Received 18 Jul 2012, Accepted 12 Sep 2012
First published online 13 Sep 2012

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Sub-oxide-to-metallic highly-crystalline nanowires with uniformly distributed nanopores in the 3 nm range have been synthesized by a unique combination of the plasma oxidation, re-deposition and electron-beam reduction. Electron beam exposure-controlled oxide → sub-oxide → metal transition is explained using a non-equilibrium model.

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Uroš Cvelbar
Zhiqiang Chen
Igor Levchenko
R. Michael Sheetz
Jacek B. Jasinski
Madhu Menon
Mahendra K. Sunkara
Kostya (Ken) Ostrikov

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Chemical Communications

Sub-oxide-to-metallic, uniformly-nanoporous crystalline nanowires by plasma oxidation and electron reduction

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