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Department of Chemistry and Biotechnology, Graduate School of Engineering, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656, Japan
; Fax: +81 3-5841-7263
; Tel: +81 3-5841-7261
Chem. Commun., 2012,48, 10481-10483
12 Jul 2012,
23 Aug 2012
First published online
24 Aug 2012
Inspired by the enzymatic ping-pong mechanism, we designed a novel “ping-pong polymerization”, which employs allylation and hydroformylation in an iterative and alternating manner. Thus, alternating and regioregular vinyl alcohol–vinyl monomer copolymers possessing multiple hydroxy groups in a periodical manner were successfully synthesized.
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