Ru complexes of thienyl-functionalized dipyrrins as NCS-free sensitizers for the dye-sensitized solar cell

Guocan Li; Paolo G. Bomben; Kiyoshi C. D. Robson; Serge I. Gorelsky; Curtis P. Berlinguette; Michael Shatruk

doi:10.1039/C2CC34311H

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Chemical Communications

Issue 70, 2012

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Ru complexes of thienyl-functionalized dipyrrins as NCS-free sensitizers for the dye-sensitized solar cell

Guocan Li,^a Paolo G. Bomben,^b Kiyoshi C. D. Robson,^b Serge I. Gorelsky,*^c Curtis P. Berlinguette*^b and Michael Shatruk*^a

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Department of Chemistry and Biochemistry, Florida State University, Tallahassee, USA
E-mail: shatruk@chem.fsu.edu ;
Fax: +1 850 644 8281 ;
Tel: +1 850 417 8417

Department of Chemistry, and the Centre for Advanced Solar Materials, University of Calgary, Calgary AB, Canada
E-mail: cberling@ucalgary.ca ;
Fax: +1 403 289 9488 ;
Tel: +1 403 220 3856

Centre for Catalysis Research and Innovation, Department of Chemistry, University of Ottawa, Ottawa, Canada
E-mail: sgorelsk@uottawa.ca ;
Fax: +1 613 562 5170 ;
Tel: +1 613 562 5800

Chem. Commun., 2012,48, 8790-8792

DOI: 10.1039/C2CC34311H
Received 03 May 2012, Accepted 09 Jul 2012
First published online 11 Jul 2012

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We report the first case of Ru(II) dipyrrinates employed as dyes in dye-sensitized solar cells. These complexes exhibit panchromatic light harvesting that results in significant DSSC current densities, rendering them promising for photovoltaic applications. Adjustment of the lowest excited state energy is required to boost the power conversion efficiency.

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Guocan Li
Paolo G. Bomben
Kiyoshi C. D. Robson
Serge I. Gorelsky
Curtis P. Berlinguette
Michael Shatruk

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