Large enhancement of single molecule fluorescence by coupling to hollow silver nanoshells

Yi Fu; Jian Zhang; Joseph R. Lakowicz

doi:10.1039/C2CC34025A

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Chemical Communications

Issue 78, 2012

Urgent high quality communications from across the chemical sciences.

Impact Factor 6.169 100 Issues per Year Indexed in MEDLINE

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Large enhancement of single molecule fluorescence by coupling to hollow silver nanoshells

Yi Fu,*^a Jian Zhang^a and Joseph R. Lakowicz^a

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Department of Molecular Biology and Biochemistry, University of Maryland School of Medicine, 725 W. Lombard Street, Baltimore, USA
E-mail: yfu@umaryland.edu

Chem. Commun., 2012,48, 9726-9728

DOI: 10.1039/C2CC34025A
Received 05 Jun 2012, Accepted 11 Aug 2012
First published online 13 Aug 2012

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Abstract
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We investigated the effect of plasmon-enhanced fluorescence using hollow silver nanoshells and observed enhancement of a single probe's fluorescence up to a factor of 3 orders of magnitude. The enhancement of the quantum efficiency is attributed to enhanced absorption and increased radiative decay rate.

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