Controlled synthesis of novel Au@MIL-100(Fe) core–shell nanoparticles with enhanced catalytic performance

Fei Ke; Junfa Zhu; Ling-Guang Qiu; Xia Jiang

doi:10.1039/C2CC33964A

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Chemical Communications

Issue 13, 2013

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Controlled synthesis of novel Au@MIL-100(Fe) core–shell nanoparticles with enhanced catalytic performance

Fei Ke,^a^b Junfa Zhu,*^a^b Ling-Guang Qiu*^c and Xia Jiang^c

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National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei 230029, P.R. China

Department of Chemical Physics, University of Science and Technology of China, Hefei 230026, P.R. China
E-mail: jfzhu@ustc.edu.cn ;
Fax: +86 551 5141078

Laboratory of Advanced Porous Materials, School of Chemistry and Chemical Engineering, Anhui University, Hefei 230039, P.R. China
E-mail: lgqiu@ahu.edu.cn ;
Fax: +86 551 5108212

Chem. Commun., 2013,49, 1267-1269

DOI: 10.1039/C2CC33964A
Received 02 Jun 2012, Accepted 27 Oct 2012
First published online 29 Oct 2012

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A novel porous Au@MIL-100(Fe) core–shell nanocatalyst with controllable MIL-100(Fe) shell thickness has been fabricated by using a versatile step-by-step fashion. Catalytic studies show that the Au@MIL-100(Fe) nanocatalyst exhibits much higher catalytic activity than the pure Au nanoparticles, suggesting that the MIL-100(Fe) shell enhances the catalytic activity via a synergistic effect.

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