Photocatalytic hydrogen evolution through fully conjugated poly(azomethine) networks

Matthias Georg Schwab; Manuel Hamburger; Xinliang Feng; Jie Shu; Hans Wolfgang Spiess; Xinchen Wang; Markus Antonietti; Klaus Müllen

doi:10.1039/C0CC04057F

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Chemical Communications

Issue 47, 2010

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Photocatalytic hydrogen evolution through fully conjugated poly(azomethine) networks

Matthias Georg Schwab,^a Manuel Hamburger,^a Xinliang Feng,^a Jie Shu,^a Hans Wolfgang Spiess,^a Xinchen Wang,*^b Markus Antonietti^b and Klaus Müllen*^a

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Max-Planck-Institute for Polymer Research, Ackermannweg 10, D-55128 Mainz, Germany
E-mail: muellen@mpip-mainz.mpg.de ;
Fax: +49 6131-379100 ;
Tel: +49 6131-379151

Max Planck Institute of Colloids and Interfaces, Research Campus Golm, D-14424 Potsdam, Germany
E-mail: xinchen.wang@mpikg.mpg.de

Chem. Commun., 2010,46, 8932-8934

DOI: 10.1039/C0CC04057F
Received 24 Sep 2010, Accepted 13 Oct 2010
First published online 02 Nov 2010

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Abstract
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Three-dimensional conjugated poly(azomethine) networks were found to be promising candidates for applications in photocatalytic water splitting. Straightforward synthetic protocols lead to fully organic photocatalysts that showed enhanced long-time stability. Furthermore, the catalytic performance of these materials was correlated to the molecular composition and the optoelectronic properties of the samples.

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Synthetic protocols, elemental analysis, FTIR and SSNMR data, DFT calculation details, SSUV and TGA data
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Matthias Georg Schwab
Manuel Hamburger
Xinliang Feng
Jie Shu
Hans Wolfgang Spiess
Xinchen Wang
Markus Antonietti
Klaus Müllen

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