Unique metabolites of Pestalotiopsis fici suggest a biosynthetic hypothesis involving a Diels–Alder reaction and then mechanistic diversification

Ling Liu; Shubin Niu; Xinhua Lu; Xulin Chen; Hua Zhang; Liangdong Guo; Yongsheng Che

doi:10.1039/B918330B

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Chemical Communications

Issue 3, 2010

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Unique metabolites of Pestalotiopsis fici suggest a biosynthetic hypothesis involving a Diels–Alder reaction and then mechanistic diversification

Ling Liu , Shubin Niu , Xinhua Lu , Xulin Chen , Hua Zhang , Liangdong Guo and Yongsheng Che

Chem. Commun., 2010, 46, 460-462

DOI: 10.1039/B918330B
Received 17 Sep 2009, Accepted 23 Oct 2009
First published on the web 13 Nov 2009

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Chloropupukeanolides A (1) and B (2), unprecedented spiroketal peroxides, and chloropupukeanone A (3), three highly functionalized metabolites featuring a chlorinated pupukeanane core, were isolated from an endophytic fungus Pestalotiopsis fici, with 1 showing significant anti-HIV-1 and cytotoxic effects.

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Ling Liu
Shubin Niu
Xinhua Lu
Xulin Chen
Hua Zhang
Liangdong Guo
Yongsheng Che

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Chemical Communications

Unique metabolites of Pestalotiopsis fici suggest a biosynthetic hypothesis involving a Diels–Alder reaction and then mechanistic diversification

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