Neutron flow-mapping: Multiscale modelling opens a new experimental window

Tom C. B. McLeish; Nigel Clarke; Eduardo de Luca; Lian R. Hutchings; Richard S. Graham; Tim Gough; Isabelle Grillo; Christine M. Fernyhough; Pierre Chambon

doi:10.1039/B916288G

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Soft Matter

Issue 22, 2009

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Neutron flow-mapping: Multiscale modelling opens a new experimental window

Tom C. B. McLeish , Nigel Clarke , Eduardo de Luca , Lian R. Hutchings , Richard S. Graham , Tim Gough , Isabelle Grillo , Christine M. Fernyhough and Pierre Chambon

Soft Matter, 2009, 5, 4426-4432

DOI: 10.1039/B916288G
Received 06 Aug 2009, Accepted 01 Sep 2009
First published on the web 22 Sep 2009
This article is part of the collection: Modelling of Soft Matter

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Small-angle neutron scattering (SANS) has delivered significant insight into the rich and varied phenomena seen in the non-linear dynamics of entangled polymers. The lengthscales accessible by SANS are ideally matched to the strongly lengthscale-dependent relaxation in entangled polymers. This, in turn, has facilitated a detailed and challenging test for models of molecular rheology. Here, we review experimental techniques, along with the multiscale modelling required to predict these measurements. This approach has enriched our understanding of monodisperse linear polymers, model linear–linear blends and branched polymers. We also indicate potential future directions for this fruitful approach.

Articles By

Tom C. B. McLeish
Nigel Clarke
Eduardo de Luca
Lian R. Hutchings
Richard S. Graham
Tim Gough
Isabelle Grillo
Christine M. Fernyhough
Pierre Chambon

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Soft Matter

Neutron flow-mapping: Multiscale modelling opens a new experimental window

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