The enantioselective intramolecular aminative functionalization of unactivated alkenes, dienes, allenes and alkynes for the synthesis of chiral nitrogen heterocycles

Sherry R. Chemler

doi:10.1039/B907743J

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Organic & Biomolecular Chemistry

Issue 15, 2009

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The enantioselective intramolecular aminative functionalization of unactivated alkenes, dienes, allenes and alkynes for the synthesis of chiral nitrogen heterocycles

Sherry R. Chemler

Org. Biomol. Chem., 2009, 7, 3009-3019

DOI: 10.1039/B907743J
Received 17 Apr 2009, First published on the web 18 Jun 2009

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The enantioselective intramolecular aminative functionalization of unactivated alkenes and related π-systems is a straight-forward and atom economical strategy for the synthesis of chiral nitrogen heterocycles. These reactions can be categorized as oxidatively neutral, such as alkene hydroamination, or as oxidative reactions, such as alkene difunctionalization, e.g. aminooxygenation and carboamination. This perspective reviews the current work in the field and explores mechanistic trends that are common among the different catalysts and reaction types.

Abstract from Catalysts & Catalysed Reactions 2009

A review, with 49 references, detailing the synthesis of chiral nitrogen heterocycles from the amination of unsaturated bonds using a wide variety of catalysts.

Abstract from Methods in Organic Synthesis 2009

A review, with 49 references, describing the synthesis of chiral nitrogen heterocycles through the intramolecular amination of unsaturated bonds using a range of different catalysts.

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Organic & Biomolecular Chemistry

The enantioselective intramolecular aminative functionalization of unactivated alkenes, dienes, allenes and alkynes for the synthesis of chiral nitrogen heterocycles

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