Reductive dearomatization of a substituted benzene triggered by a strong oxidant

Runyu Tan; Datong Song

doi:10.1039/B919233F

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Dalton Transactions

Issue 44, 2009

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Reductive dearomatization of a substituted benzene triggered by a strong oxidant

Runyu Tan and Datong Song

Dalton Trans., 2009, 9892-9897

DOI: 10.1039/B919233F
Received 16 Sep 2009, Accepted 18 Sep 2009
First published on the web 06 Oct 2009

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Two new dinuclear platinum complexes Pt₂Ph₄L^Et (1a) and Pt₂Ph₄L^F (1b) (where L^Et is 1,2,4,5-tetrakis(6-ethylquinolin-8-yl)benzene and L^F is 1,2,4,5-tetrakis(6-trifluoromethoxylquinolin-8-yl)benzene) were synthesized and characterized. Triggered by an oxidant NCS, 1a and 1b displayed interesting reactivity of reductive dearomatization of the central phenyl rings of L^Et and L^F ligands respectively. The preliminary radical scavenger test gave some mechanistic insights.

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Dalton Transactions

Reductive dearomatization of a substituted benzene triggered by a strong oxidant

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