Direct observation of a carbonylation reaction relevant to CO/alkene copolymerization in a methylpalladium carbonyl complex containing a bis(N-heterocyclic carbene) ligand

Sri S. Subramanium; LeGrande M. Slaughter

doi:10.1039/B908689G

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Dalton Transactions

Issue 35, 2009

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Direct observation of a carbonylation reaction relevant to CO/alkene copolymerization in a methylpalladium carbonyl complex containing a bis(N-heterocyclic carbene) ligand

Sri S. Subramanium and LeGrande M. Slaughter

Dalton Trans., 2009, 6930-6933

DOI: 10.1039/B908689G
Received 01 May 2009, Accepted 02 Jul 2009
First published on the web 10 Jul 2009
This article is part of the collection: N-heterocyclic carbenes

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Use of a bulky bidentate bis(NHC) ligand allows isolation of a stable cationic methylpalladium carbonyl complex that undergoes clean carbonylation to an acyl complex under excess CO, modeling a key step in CO/alkene copolymerization.

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Dalton Transactions

Direct observation of a carbonylation reaction relevant to CO/alkene copolymerization in a methylpalladium carbonyl complex containing a bis(N-heterocyclic carbene) ligand

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