Enantioselective catalysis and complexity generation from allenoates

Bryan J. Cowen; Scott J. Miller

doi:10.1039/B816700C

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Chemical Society Reviews

Issue 11, 2009

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Enantioselective catalysis and complexity generation from allenoates

Bryan J. Cowen and Scott J. Miller

Chem. Soc. Rev., 2009, 38, 3102-3116

DOI: 10.1039/B816700C
Received 01 Jun 2009, First published on the web 24 Jul 2009
This article is part of the collection: Rapid complexity generation in natural product total synthesis

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Abstract
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Lewis base catalysis of reactions with allenoates using phosphine and amine nucleophiles has emerged as a key platform for the generation of molecular complexity. Investigations in this area have established a range of suitable coupling partners for allenoates, including electron-deficient olefins, imines, and aldehydes. This tutorial review will describe these methodologies, with a special emphasis on recent work regarding asymmetric reactions using chiral Lewis base catalysts.

Abstract from Catalysts & Catalysed Reactions 2010

A review, with 56 references, describing the methodologies used for reactions with allenoates using Lewis base catalysts.

Abstract from Methods in Organic Synthesis 2010

A review, with 56 references, describing the methodologies used for reactions with allenoates using Lewis base catalysts such as phosphines and amines. Special emphasis is given to recent work using chiral Lewis base catalysts for asymmetric synthesis.

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