Detection of complex formation and determination of intermolecular geometry through electrical anharmonic coupling of molecular vibrations using electron-vibration–vibration two-dimensional infrared spectroscopy

Rui Guo; Frederic Fournier; Paul M. Donaldson; Elizabeth M. Gardner; Ian R. Gould; David R. Klug

doi:10.1039/B910804A

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Physical Chemistry Chemical Physics

Issue 38, 2009

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Detection of complex formation and determination of intermolecular geometry through electrical anharmonic coupling of molecular vibrations using electron-vibration–vibration two-dimensional infrared spectroscopy

Rui Guo , Frederic Fournier , Paul M. Donaldson , Elizabeth M. Gardner , Ian R. Gould and David R. Klug

Phys. Chem. Chem. Phys., 2009, 11, 8417-8421

DOI: 10.1039/B910804A
Received 02 Jun 2009, Accepted 08 Jul 2009
First published on the web 22 Jul 2009

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Abstract
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Electrical interactions between molecular vibrations can be non-linear and thereby produce intermolecular coupling even in the absence of a chemical bond. We use this fact to detect the formation of an intermolecular complex using electron-vibration–vibration two-dimensional infrared spectroscopy (EVV 2DIR) and also to determine the distance and angle between the two molecular species.

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Rui Guo
Frederic Fournier
Paul M. Donaldson
Elizabeth M. Gardner
Ian R. Gould
David R. Klug

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Physical Chemistry Chemical Physics

Detection of complex formation and determination of intermolecular geometry through electrical anharmonic coupling of molecular vibrations using electron-vibration–vibration two-dimensional infrared spectroscopy

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