Shedding light on water structure at air–aqueous interfaces: ions, lipids, and hydration

Heather C. Allen; Nadia N. Casillas-Ituarte; M. Roxana Sierra-Hernández; Xiangke Chen; Cheng Y. Tang

doi:10.1039/B901209E

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Physical Chemistry Chemical Physics

Issue 27, 2009

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Shedding light on water structure at air–aqueous interfaces: ions, lipids, and hydration

Heather C. Allen , Nadia N. Casillas-Ituarte , M. Roxana Sierra-Hernández , Xiangke Chen and Cheng Y. Tang

Phys. Chem. Chem. Phys., 2009, 11, 5538-5549

DOI: 10.1039/B901209E
Received 20 Jan 2009, Accepted 24 Mar 2009
First published on the web 15 May 2009

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An account is given of the current state of understanding of aqueous salt, acid, and lipid/water surfaces, interfacial depth, and molecular organization within the air–solution interfacial region. Water structure, hydration, surface propensity of solutes, and surface organization are discussed. In this perspective, vibrational sum frequency generation spectroscopic studies of aqueous surfaces are interpreted. Comment on future directions within the field of aqueous surface structure is provided.

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Heather C. Allen
Nadia N. Casillas-Ituarte
M. Roxana Sierra-Hernández
Xiangke Chen
Cheng Y. Tang

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Physical Chemistry Chemical Physics

Shedding light on water structure at air–aqueous interfaces: ions, lipids, and hydration

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