Synthetic autocatalysts show organocatalysis of other reactions

Seiji Kamioka; Dariush Ajami; Julius Rebek Jr.

doi:10.1039/B916836B

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Chemical Communications

Issue 47, 2009

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Synthetic autocatalysts show organocatalysis of other reactions

Seiji Kamioka , Dariush Ajami and Julius Rebek Jr.

Chem. Commun., 2009, 7324-7326

DOI: 10.1039/B916836B
Received 14 Aug 2009, Accepted 16 Oct 2009
First published on the web 02 Nov 2009

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Abstract
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A molecule capable of both autocatalysis and organocatalysis was synthesized. The autocatalytic activity results from the self-complementary recognition sites provided by hydrogen bonding between heterocyclic subunits and the organocatalysis resides in an embedded thiourea function. The behavior of the molecule suggests both replication and metabolism can be engineered into synthetic compounds.

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Synthesis of 2a, b, 5 and substrates and characterization byspectroscopic data
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Chemical Communications

Synthetic autocatalysts show organocatalysis of other reactions

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