Asymmetric construction of quaternary stereocenters by direct organocatalytic amination of 3-substituted oxindoles

Zi-Qing Qian; Feng Zhou; Tai-Ping Du; Bo-Lun Wang; Miao Ding; Xiao-Li Zhao; Jian Zhou

doi:10.1039/B915257A

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Chemical Communications

Issue 44, 2009

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Asymmetric construction of quaternary stereocenters by direct organocatalytic amination of 3-substituted oxindoles

Zi-Qing Qian , Feng Zhou , Tai-Ping Du , Bo-Lun Wang , Miao Ding , Xiao-Li Zhao and Jian Zhou

Chem. Commun., 2009, 6753-6755

DOI: 10.1039/B915257A
Received 27 Jul 2009, Accepted 10 Sep 2009
First published on the web 25 Sep 2009

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Quinidine derivative (QD)₂PYR was found to catalyze the asymmetric direct amination of unprotected prochiral 3-oxindole with DIAD to construct quaternary stereocenters at the C3 position with excellent enantioselectivity.

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Abstract from Methods in Organic Synthesis 2010

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Zi-Qing Qian
Feng Zhou
Tai-Ping Du
Bo-Lun Wang
Miao Ding
Xiao-Li Zhao
Jian Zhou

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Chemical Communications

Asymmetric construction of quaternary stereocenters by direct organocatalytic amination of 3-substituted oxindoles

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