The regioselective photochemical rearrangement of α-[PNtBu]4

Henrike Bladt; Silvia Gonzalez Calera; Jonathan M. Goodman; Robert J. Less; Vesal Naseri; Alexander Steiner; Dominic S. Wright

doi:10.1039/B914370J

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Chemical Communications

Issue 43, 2009

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The regioselective photochemical rearrangement of α-[PN^tBu]₄

Henrike Bladt , Silvia Gonzalez Calera , Jonathan M. Goodman , Robert J. Less , Vesal Naseri , Alexander Steiner and Dominic S. Wright

Chem. Commun., 2009, 6637-6639

DOI: 10.1039/B914370J
Received 16 Jul 2009, Accepted 07 Sep 2009
First published on the web 25 Sep 2009

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Abstract
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The photochemical dyotropic (two-bond shift) rearrangement of the phosphazane cage α-[PN^tBu]₄ (1α) into the isomer β-[PN^tBu]₄ (1β) occurs via a multi-step radical mechanism; the structures of the α and β isomers are directly analogous to isovalent α- and β-As₄S₄ and P₄S₄.

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Henrike Bladt
Silvia Gonzalez Calera
Jonathan M. Goodman
Robert J. Less
Vesal Naseri
Alexander Steiner
Dominic S. Wright

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Chemical Communications

The regioselective photochemical rearrangement of α-[PN^tBu]₄

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