Multiple convergence in polyketide biosynthesis: a third folding mode to the anthraquinone chrysophanol

Gerhard Bringmann; Tobias A. M. Gulder; Andreas Hamm; Michael Goodfellow; Hans-Peter Fiedler

doi:10.1039/B910501H

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Chemical Communications

Issue 44, 2009

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Multiple convergence in polyketide biosynthesis: a third folding mode to the anthraquinone chrysophanol

Gerhard Bringmann , Tobias A. M. Gulder , Andreas Hamm , Michael Goodfellow and Hans-Peter Fiedler

Chem. Commun., 2009, 6810-6812

DOI: 10.1039/B910501H
Received 28 May 2009, Accepted 17 Sep 2009
First published on the web 05 Oct 2009

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The polyketide chrysophanol is shown to be formed, in an organism-specific way, by a third folding mode, involving a remarkable cyclization of a bicyclic diketo precursor, thus establishing the first example of multiple convergence in polyketide biosynthesis.

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Gerhard Bringmann
Tobias A. M. Gulder
Andreas Hamm
Michael Goodfellow
Hans-Peter Fiedler

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Chemical Communications

Multiple convergence in polyketide biosynthesis: a third folding mode to the anthraquinone chrysophanol

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