Electronic and steric tuning of chiral diene ligands for rhodium-catalyzed asymmetric arylation of imines

Kazuhiro Okamoto; Tamio Hayashi; Viresh H. Rawal

doi:10.1039/B904624K

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Chemical Communications

Issue 32, 2009

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Electronic and steric tuning of chiral diene ligands for rhodium-catalyzed asymmetric arylation of imines

Kazuhiro Okamoto , Tamio Hayashi and Viresh H. Rawal

Chem. Commun., 2009, 4815-4817

DOI: 10.1039/B904624K
Received 06 Mar 2009, Accepted 24 Apr 2009
First published on the web 19 May 2009
This article is part of the collection: Selective Catalysis for Organic Synthesis

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Abstract
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Rhodium-catalyzed asymmetric arylation of imines using electronically and sterically-modified chiral diene ligands gave the corresponding diarylmethylamines in high yield and with high enantioselectivity using just 0.3 mol% of catalyst.

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Supplementary Info

Experimental procedures, compound characterization data, andX-ray crystallographic data of Rh(acac)((R)-1a)
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Crystal structure data
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Chemical Communications

Electronic and steric tuning of chiral diene ligands for rhodium-catalyzed asymmetric arylation of imines

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