Recent advancements and challenges of palladiumII-catalyzed oxidation reactions with molecular oxygen as the sole oxidant

Keith M. Gligorich; Matthew S. Sigman

doi:10.1039/B902868D

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Chemical Communications

Issue 26, 2009

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Recent advancements and challenges of palladium^II-catalyzed oxidation reactions with molecular oxygen as the sole oxidant

Keith M. Gligorich and Matthew S. Sigman

Chem. Commun., 2009, 3854-3867

DOI: 10.1039/B902868D
Received 11 Feb 2009, Accepted 30 Mar 2009
First published on the web 14 May 2009

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During the past 10 years there have been significant advances in Pd^II-catalyzed oxidation reactions where the use of ligands has led to the development of catalytic systems capable of achieving high turnover numbers, which employ molecular oxygen as the sole stoichiometric oxidant. This Feature article will highlight some of the recent developments in direct molecular oxygen-coupled Pd^II-catalyzed oxidation reactions with an emphasis on enhanced catalytic systems and new reactions. Additionally, limitations of current catalytic systems, such as ligand oxidation, are presented and their implications for the development of new reactions are discussed.

Abstract from Catalysts & Catalysed Reactions 2009

A review, with 66 references, of recent developments in palladium-catalyzed oxidation reactions which use molecular oxygen as the oxidant in so-called oxidase type reactions.

Abstract from Methods in Organic Synthesis 2009

A review, with 66 references, of recent developments in palladium-catalyzed oxidation reactions which use molecular oxygen as the oxidant, including alcohol oxidation, Heck, Wacker, homocoupling and so-called palladium oxidase reactions.

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Chemical Communications

Recent advancements and challenges of palladium^II-catalyzed oxidation reactions with molecular oxygen as the sole oxidant

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