Double-strand DNA cleavage from photodecarboxylation of (μ-oxo)diiron(III) L-histidine complex in visible light

Mithun Roy; Tuhin Bhowmick; Suryanarayanarao Ramakumar; Munirathinam Nethaji; Akhil R. Chakravarty

doi:10.1039/B802533A

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Dalton Transactions

Issue 27, 2008

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Double-strand DNA cleavage from photodecarboxylation of (μ-oxo)diiron(III) L-histidine complex in visible light

Mithun Roy , Tuhin Bhowmick , Suryanarayanarao Ramakumar , Munirathinam Nethaji and Akhil R. Chakravarty

Dalton Trans., 2008, 3542-3545

DOI: 10.1039/B802533A
Received 13 Feb 2008, Accepted 02 May 2008
First published on the web 23 May 2008

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The oxo-bridged diiron(III) complex [{Fe(L-his)(dpq)}₂(μ-O)]²⁺ having L-histidine (L-his) and dipyrido[3,2-d:2′,3′-f]quinoxaline (dpq) bound to Fe(III) exemplifies an iron-based model photonuclease that shows visible light-induced DNA double-strand cleavage in a photodecarboxylation pathway and models iron–bleomycin activity.

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Mithun Roy
Tuhin Bhowmick
Suryanarayanarao Ramakumar
Munirathinam Nethaji
Akhil R. Chakravarty

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Dalton Transactions

Double-strand DNA cleavage from photodecarboxylation of (μ-oxo)diiron(III) L-histidine complex in visible light

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