Molecular recognition in a heteromolecular radical pair system with complementary multipoint hydrogen-bonding

Hidenori Murata; Paul M. Lahti; Safo Aboaku

doi:10.1039/B800779A

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Chemical Communications

Issue 29, 2008

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Molecular recognition in a heteromolecular radical pair system with complementary multipoint hydrogen-bonding

Hidenori Murata , Paul M. Lahti and Safo Aboaku

Chem. Commun., 2008, 3441-3443

DOI: 10.1039/B800779A
Received 22 Jan 2008, Accepted 22 Apr 2008
First published on the web 02 Jun 2008

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Abstract
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Stable radicals 2-(6-uradinyl)-4,4,5,5-tetramethyl-4,5-dihydro-1H-imidazole-1-oxyl (Ur6IN) and 4-(p-tert-butylaminoxylphenyl)-2,6-di(propylamido)pyridine (DAPPN) form heterospin radical pair complexes due to complementary multi-point hydrogen-bonds.

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Supplementary Info

Synthesis, EPR, MS, computed spin densities of DAPPN, ESI-MS of Ur6IN· DAPPN and a spin density map of the Ur6IN· DAPPN model
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Chemical Communications

Molecular recognition in a heteromolecular radical pair system with complementary multipoint hydrogen-bonding

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