Regioselective 12CO/13CO exchange activity of a mixed-valent Fe(II)Fe(I) model of the Hox state of [FeFe]-hydrogenase

Christine M. Thomas; Tianbiao Liu; Michael B. Hall; Marcetta Y. Darensbourg

doi:10.1039/B719559A

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Chemical Communications

Issue 13, 2008

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Regioselective ¹²CO/¹³CO exchange activity of a mixed-valent Fe(II)Fe(I) model of the H_ox state of [FeFe]-hydrogenase

Christine M. Thomas , Tianbiao Liu , Michael B. Hall and Marcetta Y. Darensbourg

Chem. Commun., 2008, 1563-1565

DOI: 10.1039/B719559A
Received 20 Dec 2007, Accepted 23 Jan 2008
First published on the web 20 Feb 2008

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A mixed-valent Fe(II)Fe(I) model of the H_ox state of [FeFe]-hydrogenase is shown, under certain conditions, to exhibit regioselective ¹²CO/¹³CO exchange activity similar to that observed for H_ox.

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Detailed experimental procedures, and additional information about the DFT frequency calculations for 1 +
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Chemical Communications

Regioselective ¹²CO/¹³CO exchange activity of a mixed-valent Fe(II)Fe(I) model of the H_ox state of [FeFe]-hydrogenase

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