Simple dimer containing dissociatively stable mono-imidazole ligated ferrohemes

Qing-Zheng Yang; Daria Khvostichenko; John D. Atkinson; Roman Boulatov

doi:10.1039/B717858A

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Chemical Communications

Issue 8, 2008

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Simple dimer containing dissociatively stable mono-imidazole ligated ferrohemes

Qing-Zheng Yang , Daria Khvostichenko , John D. Atkinson and Roman Boulatov

Chem. Commun., 2008, 963-965

DOI: 10.1039/B717858A
Received 19 Nov 2007, Accepted 12 Dec 2007
First published on the web 04 Jan 2008

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Abstract
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In weakly coordinating solvents Fe^II meso-(N-methylimidazol-2-yl)porphine 1Fe exists as a stable dimer (K_d = 50 ± 30 nM) that binds ligands without undergoing dissociation and is presently the simplest complex in which the mono-imidazole ligation of a ferroheme is enforced without excess imidazole in solution.

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Details of syntheses, characterization, spectrophotometric titrations and computational studies
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Chemical Communications

Simple dimer containing dissociatively stable mono-imidazole ligated ferrohemes

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