Hydrogen storage in metal–organic frameworks

David J. Collins; Hong-Cai Zhou

doi:10.1039/B702858J

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Journal of Materials Chemistry

Issue 30, 2007

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Hydrogen storage in metal–organic frameworks

David J. Collins and Hong-Cai Zhou

J. Mater. Chem., 2007, 17, 3154-3160

DOI: 10.1039/B702858J
Received 26 Feb 2007, Accepted 21 Mar 2007
First published on the web 11 Apr 2007
This article is part of the collection: New energy materials

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For any potential hydrogen-storage system, raw uptake capacity must be balanced with the kinetics and thermodynamics of uptake and release. Metal–organic frameworks (MOFs) provide unique systems with large overall pore volumes and surface areas, adjustable pore sizes, and tunable framework–adsorbate interaction by ligand functionalization and metal choice. These remarkable materials can potentially fill the niche between other physisorbents such as activated carbon, which have similar uptake at low temperatures but low affinity for hydrogen at ambient temperature, and chemical sorbents such as hydrides, which have high hydrogen uptakes but undesirable release kinetics and thermodynamics.

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Hydrogen storage in metal–organic frameworks

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