η1-2-Pyrone metal carbonyl complexes as CO-releasing molecules (CO-RMs): A delicate balance between stability and CO liberation

Ian J. S. Fairlamb; Jason M. Lynam; Benjamin E. Moulton; Ian E. Taylor; Anne K. Duhme-Klair; Philip Sawle; Roberto Motterlini

doi:10.1039/B707377A

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Dalton Transactions

Issue 33, 2007

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η¹-2-Pyrone metal carbonyl complexes as CO-releasing molecules (CO-RMs): A delicate balance between stability and CO liberation

Ian J. S. Fairlamb , Jason M. Lynam , Benjamin E. Moulton , Ian E. Taylor , Anne K. Duhme-Klair , Philip Sawle and Roberto Motterlini

Dalton Trans., 2007, 3603-3605

DOI: 10.1039/B707377A
Received 16 May 2007, Accepted 01 Jun 2007
First published on the web 29 Jun 2007

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Abstract
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An evaluation of the CO releasing ability of iron(II) and molybdenum(II) complexes has facilitated the discovery of the most rapid CO releaser, namely [Mo(CO)₃(η⁵-C₅H₅)(η¹-{O}–C{ [double bond, length as m-dash] O}–O–CMeCH-COMeCBr)]BF₄ (CORM-F10), reported to date. The rate of CO release is related to the overall solution phase stability of the transition metal carbonyl complex. The cytotoxity and vasodilatory properties of CORM-F10 have been determined.

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Ian J. S. Fairlamb
Jason M. Lynam
Benjamin E. Moulton
Ian E. Taylor
Anne K. Duhme-Klair
Philip Sawle
Roberto Motterlini

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Dalton Transactions

η¹-2-Pyrone metal carbonyl complexes as CO-releasing molecules (CO-RMs): A delicate balance between stability and CO liberation

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