Oxygen-17 hyperfine structures in the pure rotational spectra of SrO, SnO, BaO, HfO and ThO

Christopher T. Dewberry; Kerry C. Etchison; Garry S. Grubbs II; Robert A. Powoski; Michal M. Serafin; Sean A. Peebles; Stephen A. Cooke

doi:10.1039/B712798G

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Physical Chemistry Chemical Physics

Issue 44, 2007

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Oxygen-17 hyperfine structures in the pure rotational spectra of SrO, SnO, BaO, HfO and ThO

Christopher T. Dewberry , Kerry C. Etchison , Garry S. Grubbs II , Robert A. Powoski , Michal M. Serafin , Sean A. Peebles and Stephen A. Cooke

Phys. Chem. Chem. Phys., 2007, 9, 5897-5901

DOI: 10.1039/B712798G
Received 20 Aug 2007, Accepted 26 Sep 2007
First published on the web 09 Oct 2007

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Hyperfine structures arising from the couplings of the nuclear spin angular momentum of ¹⁷O (I = 5/2) with the end over end rotation of several metal-containing diatomic monoxides have been observed using a Fourier transform microwave spectrometer. The molecules have been produced by reacting ¹⁷O₂ with laser ablated metal atoms. The oxygen-17 nuclear quadrupole coupling constants have been determined for the title molecules and are interpreted in terms of a simple Townes–Dailey model. Also, the oxygen-17 nuclear spin-rotation constants have been determined and used to calculate the oxygen-17 shieldings for each molecule.

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Christopher T. Dewberry
Kerry C. Etchison
Garry S. Grubbs II
Robert A. Powoski
Michal M. Serafin
Sean A. Peebles
Stephen A. Cooke

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Physical Chemistry Chemical Physics

Oxygen-17 hyperfine structures in the pure rotational spectra of SrO, SnO, BaO, HfO and ThO

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