Casting a new light on azide photochemistry: photolytic production of cyclic-N3

Peter C. Samartzis; Alec M. Wodtke

doi:10.1039/B704782G

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Physical Chemistry Chemical Physics

Issue 24, 2007

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Casting a new light on azide photochemistry: photolytic production of cyclic-N₃

Peter C. Samartzis and Alec M. Wodtke

Phys. Chem. Chem. Phys., 2007, 9, 3054-3066

DOI: 10.1039/B704782G
Received 29 Mar 2007, Accepted 01 May 2007
First published on the web 23 May 2007

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Abstract
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The first postulated structure of the N₃ moiety appeared in a scientific journal in 1890 and was reported as a cyclic triangle with one N,N double bond and two N,N single bonds. Only in the last several years has our understanding of azides advanced to the point that we can now claim to know how to synthesize this prototypical bonding motif. This article examines the experiments and theory that were essential in reaching this point and suggests future directions of research on cyclic-N₃.

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Physical Chemistry Chemical Physics

Casting a new light on azide photochemistry: photolytic production of cyclic-N₃

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