Jump to main content
Jump to site search

Issue 4, 2006
Previous Article Next Article

Local and regional air pollution in Ireland during an intensive aerosol measurement campaign

Author affiliations

Abstract

An intensive two month measurement campaign has been performed during a two year study of major component composition of urban PM10 and PM2.5 in Ireland (J. Yin, A. G. Allen, R. M. Harrison, S. G. Jennings, E. Wright, M. Fitzpatrick, T. Healy, E. Barry, D. Ceburnis and D. McCusker, Atmos. Res., 2005, 78(3–4), 149–165). Measurements included size-segregated mass, soluble ions, elemental carbon (EC) distributions, fine and coarse fraction organic carbon (OC) and major gases along with standard meteorological measurements. The study revealed that urban emissions in Ireland had mainly a local character and therefore were confined within a limited area of 20–30 km radius, without significantly affecting regional air quality. Gaseous measurements have shown that urban emissions in Ireland had clear, but fairly limited influence on the regional air quality due to favorable mixing conditions at higher wind speeds, in particular from the western sector. Size-segregated mass and chemical measurements revealed a clear demarcation size between accumulation and coarse modes at about 0.8 μm which was constant at all sites. Carbonaceous compounds at the urban site accounted for up to 90% of the particle mass in a size range of 0.066–0.61 μm. Nss SO42− concentrations in PM2.5 were only slightly higher at the urban site compared to the rural or coastal sites, while NO3 and NH4+ concentrations were similar at the urban and coastal sites, but were a factor of 2 to 3 higher than at the rural site. OC was highly variable between the sites and revealed clear seasonal differences. Natural or biogenic OC component accounted for <10% in winter and up to 30% in summer of the PM2.5 OC at urban sites. A contribution of biogenic OC component to PM2.5 OC mass at rural site was dominant.

Graphical abstract: Local and regional air pollution in Ireland during an intensive aerosol measurement campaign

Back to tab navigation

Publication details

The article was received on 11 Nov 2005, accepted on 06 Mar 2006 and first published on 14 Mar 2006


Article type: Paper
DOI: 10.1039/B516029D
Citation: J. Environ. Monit., 2006,8, 479-487
  •   Request permissions

    Local and regional air pollution in Ireland during an intensive aerosol measurement campaign

    D. Ceburnis, J. Yin, A. G. Allen, S. G. Jennings, R. M. Harrison, E. Wright, M. Fitzpatrick, T. Healy and E. Barry, J. Environ. Monit., 2006, 8, 479
    DOI: 10.1039/B516029D

Search articles by author

Spotlight

Advertisements