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Mechanistic investigation of CO2 hydrogenation by Ru(II) and Ir(III) aqua complexes under acidic conditions: two catalytic systems differing in the nature of the rate determining step

Seiji Ogo,*ab   Ryota Kabe,ac   Hideki Hayashi,b   Ryosuke Haradaa and   Shunichi Fukuzumi*c  
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Corresponding authors
a
Center for Future Chemistry, Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka, Japan
E-mail: ogo-tcm@mbox.nc.kyushu-u.ac.jp
b
PRESTO, Japan Science and Technology Agency (JST), 4-1-8, Honcho, Kawaguchi, Saitama, Japan
c
Department of Material and Life Science, Division of Advanced Science and Biotechnology, Graduate School of Engineering, Osaka University, SORST, Japan Science and Technology Agency (JST), Suita, Japan
Dalton Trans., 2006, 4657-4663

DOI: 10.1039/B607993H
Received 05 Jun 2006, Accepted 01 Aug 2006
First published online 16 Aug 2006

This article is part of themed collection: Carbon dioxide at metal centres
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