Electricity from low-level H2 in still air – an ultimate test for an oxygen tolerant hydrogenase

Kylie A. Vincent; James A. Cracknell; Jeremy R. Clark; Marcus Ludwig; Oliver Lenz; Bärbel Friedrich; Fraser A. Armstrong

doi:10.1039/B614272A

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Chemical Communications

Issue 48, 2006

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Electricity from low-level H₂ in still air – an ultimate test for an oxygen tolerant hydrogenase

Kylie A. Vincent , James A. Cracknell , Jeremy R. Clark , Marcus Ludwig , Oliver Lenz , Bärbel Friedrich and Fraser A. Armstrong

Chem. Commun., 2006, 5033-5035

DOI: 10.1039/B614272A
Received 02 Oct 2006, Accepted 27 Oct 2006
First published on the web 09 Nov 2006

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We demonstrate an extreme test of O₂ tolerance for a biological hydrogen-cycling catalyst: the generation of electricity from just 3% H₂ released into still, ambient air using an open fuel cell comprising an anode modified with the unusual hydrogenase from Ralstonia metallidurans CH34, that oxidizes trace H₂ in atmospheric O₂, connected via a film of electrolyte to a cathode modified with the fungal O₂ reductase, laccase.

Articles By

Kylie A. Vincent
James A. Cracknell
Jeremy R. Clark
Marcus Ludwig
Oliver Lenz
Bärbel Friedrich
Fraser A. Armstrong

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Chemical Communications

Electricity from low-level H₂ in still air – an ultimate test for an oxygen tolerant hydrogenase

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