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Volume 115, 2000
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Towards disentangling coupled electronic–vibrational dynamics in ultrafast non-adiabatic processes

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Abstract

Femtosecond time-resolved photoelectron spectroscopy is emerging as a new technique for investigating polyatomic excited state dynamics. Due to the sensitivity of photoelectron spectroscopy to both electronic configurations and vibrational dynamics, it is well suited to the study of non-adiabatic processes such as internal conversion, which often occur on sub-picosecond time scales. We discuss the technical requirements for such experiments, including lasers systems, energy- and angle-resolved photoelectron spectrometers and new detectors for coincidence experiments. We present a few examples of these methods applied to problems in diatomic wavepacket dynamics and ultrafast non-adiabatic processes in polyatomic molecules.

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Publication details

The article was received on 10 Feb 2000 and first published on 06 Apr 2000


Article type: Paper
DOI: 10.1039/B001138J
Citation: Faraday Discuss., 2000,115, 33-48
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    Towards disentangling coupled electronic–vibrational dynamics in ultrafast non-adiabatic processes

    V. Blanchet, S. Lochbrunner, M. Schmitt, J. P. Shaffer, J. J. Larsen, M. Z. Zgierski, T. Seideman and A. Stolow, Faraday Discuss., 2000, 115, 33
    DOI: 10.1039/B001138J

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