Quantum beat spectroscopy is a Doppler-free time domain method
based on the creation of molecular coherences with a laser pulse and the
measurement of their subsequent time evolution. Fourier transformation of
the time evolution allows a spectrum in the frequency domain with lifetime-
limited resolution to be recovered. This article gives an account of the
technique applied in high resolution mode which allows the study of
isolated molecules, radicals and complexes in extensive detail and with
great accuracy.
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