Electrocatalytic four-electron reduction of oxygen to water by a highly flexible cofacial cobalt bisporphyrin

Christopher J. Chang; Yongqi Deng; Chunnian Shi; C. K. Chang; Fred C. Anson; Daniel G. Nocera

doi:10.1039/B001620I

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Chemical Communications

Issue 15, 2000

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Electrocatalytic four-electron reduction of oxygen to water by a highly flexible cofacial cobalt bisporphyrin

Christopher J. Chang , Yongqi Deng , Chunnian Shi , C. K. Chang , Fred C. Anson and Daniel G. Nocera

Chem. Commun., 2000, 1355-1356

DOI: 10.1039/B001620I
Received 16 Feb 2000, Accepted 11 Apr 2000
First published on the web 04 Jul 2000

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Dicobalt(II) cofacial bisporphyrins anchored by dibenzofuran (DPD) and xanthene (DPX) are efficient electrocatalysts for the four-electron reduction of oxygen to water despite their ca. 4 Å difference in metal–metal distances, suggesting that the considerable longitudinal ‘Pac-Man’ flexibility of the pillared platforms is the origin for the similar catalytic reactivity of these structurally disparate systems.

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Christopher J. Chang
Yongqi Deng
Chunnian Shi
C. K. Chang
Fred C. Anson
Daniel G. Nocera

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Chemical Communications

Electrocatalytic four-electron reduction of oxygen to water by a highly flexible cofacial cobalt bisporphyrin

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