FTIR-spectroscopy of molecular clusters in pulsed supersonic slit-jet expansions

Thomas Häber; Ulrich Schmitt; Martin A. Suhm

doi:10.1039/A907264K

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Physical Chemistry Chemical Physics

Issue 24, 1999

High quality research in physical chemistry, chemical physics and biophysical chemistry.

Impact Factor 3.573 48 Issues per Year Indexed in MEDLINE

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FTIR-spectroscopy of molecular clusters in pulsed supersonic slit-jet expansions

Thomas Häber, Ulrich Schmitt and Martin A. Suhm

Phys. Chem. Chem. Phys., 1999,1, 5573-5582

DOI: 10.1039/A907264K

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Abstract
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A new approach to the Fourier transform infrared (FTIR) absorption spectroscopy of molecular clusters in pulsed supersonic jets is developed to the point where it is competitive with high-sensitivity laser absorption techniques for intermediate and large molecular systems. A combination of rapid spectral acquisition and of a buffered jet chamber enables the use of intense gas pulses which cover complete interferometer scans. Applications to (N₂O)_n, (CH₃OH)_n and (HCl)_n demonstrate the capabilities of this technique. Investigations of the association of bulky alcohols and of clusters within clusters illustrate some ongoing research.

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